I'd have to say Blitz's Rocket-Hook.
Emissary of the League
A well timed Karthus Ult
Nidalee spear or Singed fling.
I assumed you'd say any ability from Singed, Sly.
well there's nothing satisfying about free wins, i meant if Singed's only ability was fling it'd be satisfying
Timmy the Spork
it's very satisfying when an enemy who would otherwise escape hits one of Teemo's shrooms.
The "SMACK" sound on mundo's cleaver makes it a very satisfying move to land.
when the other team ignores you during your kat ult.
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